J9Ö±Óª¼¯ÍÅ

J9Ö±Óª¼¯ÍÅ(Öйú´ó½)¹Ù·½ÍøÕ¾-Ó­×ÔÓÉ,´´½«À´
NEWS CENTER

ÐÂÎÅÖÐÐÄ

J9Ö±Óª¼¯ÍÅ(Öйú´ó½)¹Ù·½ÍøÕ¾-Ó­×ÔÓÉ,´´½«À´

Ñõ»¹Ô­×îÐÂ×êÑгɾͣ¡¶à¿×ÄÉÃ×Çòԭλ¹¹ÖþFe3N/FeCoÔÓ»¯Ì¼×ÊÁϸßЧµç´ß»¯!

¹¦·ò£º2022-08-29     ÆðÔ´£ºNano Research Energy

2022Äê8ÔÂ23ÈÕ £¬Ç廪´óѧÖ÷°ìµÄÄÜԴѧÊõÆÚ¿¯Nano Research Energy£¨https://www.sciopen.com/journal/2790-8119 £©±àί¡¢ÏæÌ¶´óѧÁõÒæ½­¸±½ÌÊÚ¿ÎÌâ×éÌá³öÒ»ÖÖµ¥Ò»ÓÐЧµÄԭλÔ챸Fe3NºÍFeCoÄÉÃ׿ÅÁ£½¨ÊεÄÔÓ»¯Ì¼×ÊÁϵIJ½Öè²¢ÓÃÓÚ¸ßЧÑõ»¹Ô­´ß»¯·´Ó³¡£ÂÛÎıêÌâΪ¡°Metal-coordinated porous polydopamine nanospheres derived Fe3N-FeCo encapsulated N-doped carbon as a highly efficient electrocatalyst for oxygen reduction reaction¡±¡£

202282615400320

ͼ1. (a) Fe3N-FeCo@NCµÄÔ챸ʾÒâͼ £»Fe3N-FeCo@NCµÄTEM (b)ºÍHRTEM (c)ÕÕÆ¬ £»Fe3N-FeCo@NCµÄLSVÇúÏß(d) £»»ùÓÚFe3N-FeCo@NCµÄп¿Õµç³ØµÄ¹¦ÂÊÃÜ¶È (e)¡£

Ñõ»¹Ô­·´Ó³(ORR)ÊǽðÊô¿ÕÆøµç³ØµÄ³ÁÒª°ë·´Ó³ £¬µ«ÊÇ·´Ó³¶¯Á¦Ñ§»ºÂý¡£Pt»ù´ß»¯¼ÁÄÜÓÐЧÌáÉýORR¶¯Á¦Ñ§ £¬µ«´æÔÚ²»±äÐԵ͡¢×ÊÔ´½ôȱ¡¢¼ÛÖµ°º¹óµÈÎÊÌâ £¬ÏÞ¶ÈÁ˽ðÊô¿ÕÆøµç³ØµÄóÒ×»¯ÀûÓá£Òò¶ø £¬¿ª·¢·Ç¹ó½ðÊôORR´ß»¯¼ÁÖÁ¹Ø³ÁÒª¡£ÔÚÒÑ¿ª·¢µÄ¸÷Àà·Ç¹ó½ðÊô´ß»¯¼ÁÖÐ £¬½ðÊôµª»¯Îï²ôÔÓµÄ̼×ÊÁÏ£¨MNx-C£©ÓÉÓÚÆä¸ßµ¼µçÐÔ¡¢ÓÅÒìµÄÑõ»¹Ô­´ß»¯»îÐԺ;­¼ÃºÏÓÃÐÔ±»ÒÔΪÊÇ×îÓпÉÄÜÈ¡´úPt»ù´ß»¯¼ÁµÄÒ»Àà×ÊÁÏ¡£ÆäÖÐ £¬µª»¯Ìú£¨Fe3N£©½¨ÊεÄ̼×ÊÁÏ£¨Fe3N-C£©ÓµÓпÉÓëPt/CæÇÃÀµÄORR´ß»¯»îÐÔ¡£È»¶ø £¬ÐγÉFe3N¿ÅÁ£Í¨³£±ØÒª¸ßΰ±»¯ £¬Õâ²»½öÔö³¤ÁËÔ챸³É±¾Ò²´æÔÚ°²È«Òþ»¼¡£ÈôºÎͨ¹ý·Ç¸ßΰ±»¯²½ÖèÀ´Ô챸Fe3NÄÉÃ׿ÅÁ£½¨ÊεÄ̼×ÊÁϲ¢ÏÔÖøÌáÉýÆäORR´ß»¯»îÐÔ³ÉΪÁËÐµĹØ×¢µã¡£

Òò¶ø £¬ÁõÒæ½­¿ÎÌâ×éÌá³öÒ»ÖÖµ¥Ò»ÓÐЧµÄԭλÔ챸Fe3NºÍFeCoÄÉÃ׿ÅÁ£½¨ÊεÄÔÓ»¯Ì¼×ÊÁϵIJ½Öè²¢ÓÃÓÚ¸ßЧÑõ»¹Ô­´ß»¯·´Ó³¡£Ê×ÏÈ £¬Í¨¹ýÈéÒº×é×°ºÍ×ԾۺϵIJ½ÖèÔ챸Á˶à¿×¾Û¶à°Í°·½ðÊôÄÉÃ×Çò£¨ÈçFe-PDA@Co£© £¬ËæºóÀûÓþ۶à°Í°·¡¢½ðÊôÓëÈý¾ÛÇè°·µÄÏ໥×÷ÓÃÔÚ¾Û¶à°Í°·½ðÊôÄÉÃ×Çò±í±í°ü¸²Èý¾ÛÇè°·µÃµ½Fe-PDA@Co@melamineÂçºÏÎï £¬×îºóͨ¹ý¸ßÎÂÈȽâµÃµ½Fe3NºÍFeCo½¨ÊεĶà¿×̼ÇòºÍ̼ÄÉÃׯ¬¹²´æµÄÔÓ»¯Ì¼×ÊÁÏFe3N-FeCo@NC¡£ÔÚ±¾¹¤×÷Öв»±ØÒª¾­¹ý¸ßΰ±»¯¼´¿ÉԭλÐγÉFe3NÄÉÃ׿ÅÁ£ £¬ÕâÖØÒªµÃÒæÓÚÈéÒº×é×°ºÍ×Ô¾ÛºÏÏà½áºÏµÄÕ½Êõ £¬Ê¹Ìú¾ùÔÈ·ÖÉ¢ÔÚ¾Û¶à°Í°·¶à¿×ÇòÖÐ £¬Í¬Ê±Èý¾ÛÇè°·ÓëÌúÒ²ÓÐÏ໥×÷Óà £¬Òò¶ø²»±ØÒª¶î±íµÄ¸ßΰ±»¯¡£Fe3N-FeCo@NCÓµÓнϴóµÄ±È±í±í»ýºÍ¶à¼¶¿×½á¹¹ £¬Í¬Ê±ÓµÓÐFe3N¡¢FeCo¡¢M-NxµÈ»îÐÔÖÖ £¬Òò¶øÓµÓÐÓÅÒìµÄÑõ»¹Ô­µç´ß»¯»îÐÔ¡£ÔÚ0.1M KOH½éÖÊÖÐ £¬Fe3N-FeCo@NCµÄÕØÊ¼µçλΪ1.05 V £¬°ë²¨µçλΪ0.89 V £¬³¬¹ýPt/CµÄÕØÊ¼µç루0.97 V£©ºÍ°ë²¨µç루0.85 V£© £¬Ò²Ô¶Ô¶³¬¹ý²Î±ÈÑùÆ·Fe/NC£¨ÏÈÇýÌå²»º¬CoºÍÈý¾ÛÇè°·£©ºÍFe,Co/NC£¨ÏÈÇýÌå²»º¬Èý¾ÛÇè°·£© £¬ÊÇĿǰMNx-C×ÊÁÏ ORR»úÄܵÄ×î¸ßÖµÖ®Ò»¡£´Ë±í £¬Fe3N-FeCo@NCµÄ²»±äÐԺͿ¹¼×´¼»úÄÜÒ²Ô¶Ô¶³¬¹ýPt/C¡ £»ùÓÚFe3N-FeCo@NCΪ¿ÕÆøÒõ¼«µÄп¿ÕÆøµç³ØµÄ¿ªÂ·µçѹΪ1.50 V £¬¹¦ÂÊÃܶȴï141 mW¡¤cm?2 £¬±ÈÈÝÁ¿Îª806.6 mAh¡¤g?1Zn £¬ÏÔÖø¸ßÓÚPt/C×é×°µÄµç³Ø£¨¿ªÂ·µçѹΪ1.48 V £¬¹¦ÂÊÃܶÈ113 mW¡¤cm?2 £¬±ÈÈÝÁ¿Îª660.6 mAh¡¤g?1Zn£©¡£Í¬Ê± £¬»ùÓÚFe3N-FeCo@NCµÄп¿ÕÆøµç³ØÓµÓÐÓÅÒìµÄ±¶ÂÊ»úÄܺͲ»±äÐÔ¡£ÒÔÉÏÁ˾ÖÅú×¢Fe3N-FeCo@NCÊÇÒ»ÖÖ¸ßЧÇÒ²»±äµÄORRµç´ß»¯¼Á £¬ÓÐÀûÓÚÍÆ¶¯Ð¿¿Õµç³ØµÄÏÖʵÀûÓá£

ÓйØÂÛÎÄÐÅÏ¢£º

Guo, F. J.; Zhang, M. Y.; Yi, S. C.; Li, X. X.; Xin, R.; Yang, M.; Liu, B.; Chen, H. B.; Li, H. M.; Liu, Y. J. Metal-coordinated porous polydopamine nanospheres derived Fe3N-FeCo encapsulated N-doped carbon as a highly efficient electrocatalyst for oxygen reduction reaction. Nano Res. Energy 2022, 1: e9120027. DOI: 10.26599/NRE.2022.9120027. https://doi.org/10.26599/NRE.2022.9120027 .

×÷ΪNano Researchæ¢Ãÿ¯ £¬Nano Research Energy (ISSN: 2791-0091; e-ISSN: 2790-8119; ¹ÙÍø: https://www.sciopen.com/journal/2790-8119)ÓÚ2022Äê3Ô´´¿¯ £¬ÓÉÇ廪´óѧÇúÁ¼Ìå½ÌÊÚºÍÏã¸Û³ÇÊдóѧ֧´ºÒå½ÌÊÚ¹²Í¬µ£ÈÎÖ÷±à¡£Nano Research EnergyÊÇÒ»±¾¹ú¼Ê»¯µÄ¶àѧ¿Æ½»²æ £¬È«Ó¢ÎÄÊ¢¿ª»ñÈ¡ÆÚ¿¯ £¬¾Û½¹ÄÉÃ××ÊÁϺÍÄÉÃ׿ÆÑ§¼¼ÊõÔÚÐÂÐÍÄÜÔ´ÓйØÁìÓòµÄÇ°ÑØ×êÑÐÓëÀûÓà £¬¶Ô±ê¹ú¼Ê¶¥¼¶ÄÜÔ´ÆÚ¿¯ £¬ÖÂÁ¦ÓÚ°ä·¢¸ßˮƽµÄÔ­´´ÐÔ×êÑкÍ×ÛÊöÀàÂÛÎÄ¡£2023Äê֮ǰÃâÊÕAPCÓöÈ £¬»¶Ó­¸÷λ½ÌԱӻԾͶ¸å¡£Í¶¸åÇëÁªÏµ£ºNanoResearchEnergy@tup.tsinghua.edu.cn.

¡¾ÍøÕ¾µØÍ¼¡¿
¡¾ÍøÕ¾µØÍ¼¡¿